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JAEA Reports

Distribution of actinide elements among various environmental factors (II)

Kudo, Akira*; Fujikawa, Yoko*

JNC TJ8400 2000-010, 67 Pages, 2000/02

JNC-TJ8400-2000-010.pdf:2.17MB

The first and second environmental releases of man-made $$^{239+240}$$Pu came from nuclear explosions at Alamagordo and Nagasaki in 1945. The release at Nagasaki was more serious than at Alamagordo, because it happened in an area with a high population density. Unfissioned $$^{239+240}$$Pu and various fission products have been interacting here with various environmental materials (soils, sediments, and plants) under wet and temperature conditions for more than 45 years. To assess the environmental mobility of $$^{239+240}$$Pu, the distributions of radionuclides from this release were investigated at Nishiyama where heavy black rain containing unfissioned plutonium and fission products fell 30 minutes after the nuclear explosion. The vertical distributions of $$^{137}$$Cs and $$^{239+240}$$Pu were determined in unsaturated soil cores up to 450cm deep. Most radionuclides were found in the soil column 30cm from the ground surface. However, $$^{239+240}$$Pu were detected in the groundwater as well below a depth of 200cm. No $$^{137}$$Cs was found below 40cm from the ground surface or in groundwater. These observations reveal that about 3% of the total $$^{239+240}$$Pu have been migrating in the soil at a faster rate than the remaining $$^{239+240}$$Pu. Sharp peak of $$^{137}$$Cs and $$^{239+240}$$Pu, indicating heavy deposition from the Nagasaki local fallout of 1945, were found in sediment cores collected from the Nishiyama reservoir. $$^{239+240}$$Pu peaks were unexpectedly discovered in pre-1945 sediment core sections. NO $$^{137}$$Cs was found. By contrast to the distribution in sediment cores, $$^{137}$$Cs in tree rings had spread by diffusion from the bark to the center of the tree without holding a fallout deposition record. Most of the $$^{239+240}$$Pu was distributed in the tree rings following a similar deposition record to that found in sediment cores. Furthermore, a very small amount of $$^{239+240}$$Pu (about 1%) was found unexpectedly in pre-1945 tree rings. The only reasonable ...

JAEA Reports

None

*

PNC TJ1309 96-001, 113 Pages, 1996/03

PNC-TJ1309-96-001.pdf:3.42MB

no abstracts in English

JAEA Reports

None

*; Kase, Takeshi

PNC TJ8603 92-001, 22 Pages, 1992/03

PNC-TJ8603-92-001.pdf:0.52MB

no abstracts in English

Oral presentation

Development of resonance ionization mass spectrometry of Sr isotopes, 4

Miyabe, Masabumi; Oba, Masaki; Akaoka, Katsuaki; Wakaida, Ikuo; Iwata, Yoshihiro*; Jung, K.*; Hasegawa, Shuichi*

no journal, , 

For the radioactivity evaluation regarding to the accident of TEPCO Fukushima Daiichi Nuclear Power Station, time-consuming and skills-required sample pretreatments for $$^{90}$$Sr analysis (radiometric or ICP-MS analyses) is serious issue. We are developing a ultra-sensitive and rapid analytical technique for $$^{90}$$Sr by combining resonance ionization spectroscopy, in which only the atoms of specific isotope can be ionized using the slight difference in level energy, and ion trap technique, in which only the ions of specific isotope can be trapped for a long duration to observe them with high sensitivity. In this study, we applied a continuous-wave isolated-core excitation technique (cw-ICE) for the first time to search for highly efficient and isotope-selective ionization schemes, especially for the Rydberg series converging to the 5$$p_{1/2,3/2}$$ ionic levels, of which information is quite scarce. As a result, we have revealed a detailed level-structure of autoionizing 5$$p_{1/2,3/2}$$(nl) series of Sr atoms.

Oral presentation

Development of an in-situ detection method for $$^{90}$$Sr/$$^{90}$$Y in high gamma radiation backgrounds utilizing Cherenkov radiation directivity

Terasaka, Yuta; Sato, Yuki; Furuta, Yoshihiro*; Kubo, Shin*

no journal, , 

no abstracts in English

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